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- W3136183592 abstract "Redox reactions in silicate glassmelts and glasses are considered from two end-member kinetics perspectives. Open-system redox involves long-distance (i.e. far beyond the atomic scale) chemical diffusion as the glass/melt evolves toward equilibrium with the external environment. Closed-system (or internal) redox involves relatively short-range (near-atomic-scale) chemical diffusion as the redox potentials of component cations interact, particularly during quenching. The thermodynamics involved are conceptually straightforward and are usefully considered using Ellingham-type diagrams. Practically, particularly for closed systems, the difficulty in designing or understanding redox behavior is ascertaining the activities of oxide components and their sensitivity to temperature (± pressure). Redox dynamics are strongly influenced by heterovalency, which effects electronic conductivity that decouples all ionic fluxes. The reaction morphology, though, frequently can be used to discern the redox dynamics for the case of open systems. Examples presented include float processing of glassmelts and oxidation of glasses as open systems and glassmelt fining and glass coloration as closed systems." @default.
- W3136183592 created "2021-03-29" @default.
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- W3136183592 date "2021-02-01" @default.
- W3136183592 modified "2023-09-23" @default.
- W3136183592 title "Redox Thermodynamics and Kinetics in Silicate Melts and Glasses" @default.
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- W3136183592 doi "https://doi.org/10.1002/9781118801017.ch5.6" @default.
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