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- W3136184018 abstract "Transition metal-catalyzed asymmetric transformations of alkenes and alkynes can upgrade readily available unsaturated compounds to valuable building blocks for organic synthesis. Late transition metals supported by asymmetric ligands, particularly palladium, rhodium, and iridium, have traditionally been employed for enantioselective functionalization of alkenes and alkynes, but these precious metals are costly. Silver is a much less expensive late transition metal with good Lewis acidity that can accommodate diverse ligands and coordination geometries. Silver(I) complexes are also capable of engaging in non-covalent interactions with alkenes and alkynes to drive selectivity in reactions at both the unsaturated bond, as well as at an adjacent activated allylic or propargylic C–H bond. This short review summarizes recent developments in asymmetric silver-catalyzed reactions of alkene-containing and alkyne-containing compounds. Direct enantioselective transformations of the alkene/alkyne π bond are described, as well as examples where the site of unsaturation drives functionalization at an adjacent C–H bond." @default.
- W3136184018 created "2021-03-29" @default.
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- W3136184018 creator A5063494151 @default.
- W3136184018 date "2021-08-01" @default.
- W3136184018 modified "2023-09-23" @default.
- W3136184018 title "Silver-catalyzed enantioselective functionalizations of alkenes and alkynes: A short review" @default.
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- W3136184018 doi "https://doi.org/10.1016/j.cogsc.2021.100483" @default.
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