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- W3136203881 abstract "Abstract An efficient palladium‐catalyzed N ‐arylations of 3‐aryl‐1‐tosyl‐1 H ‐pyrazol‐5‐amines with arylbromides is established. A series of diversified N ‐arylated products are obtained in excellent yields with broad substrate scope. Importantly, the N ‐arylated products undergo 1,4‐ and 1,6‐migration reactions of Ts group under the action of Cs 2 CO 3 , affording the N ‐Ts‐substituted pyrroles as major products (1,6‐migration). Similar results can also be directly obtained by palladium‐catalyzed reactions of 3‐aryl‐1‐tosyl‐1 H ‐pyrazol‐5‐amines with arylbromides in the presence of Cs 2 CO 3 as a base. Mechanistic studies reveal that the Ts‐migration is achieved through an intermolecular pathway." @default.
- W3136203881 created "2021-03-29" @default.
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- W3136203881 date "2021-04-14" @default.
- W3136203881 modified "2023-09-26" @default.
- W3136203881 title "Pd‐Catalyzed <i>N</i> ‐Arylations of 3‐Aryl‐1‐tosyl‐1 <i>H</i> ‐pyrazol‐5‐amines with Arylbromides and the Migration of Ts Group" @default.
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- W3136203881 doi "https://doi.org/10.1002/cctc.202100193" @default.
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