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• W3136234979 endingPage "261" @default.
• W3136234979 startingPage "255" @default.
• W3136234979 abstract "With a superb ability to dissolve the long-chain lithium polysulfides (Li2S4−8, LPSs) intermediates and promote the conversion between sulfur (S) and lithium sulfide (Li2S), ether-based electrolytes have been widely employed in lithium-sulfur (Li-S) batteries. While for ether-based Li-S batteries, the low reaction barrier is only overserved under superfluous electrolyte conditions. Aiming to figure out how Li-S batteries work and fail under lean-ether-electrolyte conditions, herein, we carefully simulated the internal electrolyte environment and investigated the electrochemical behavior of the ether-based Li-S batteries under the different E/S ratios (1, 2, 3, 4, 6, and 10 μL mg−1). The physicochemical and electrochemical characterizations reveal that the dissolution of the long-chain LPSs intermediates in lean ether electrolytes significantly reduces the wettability and conductivity of the electrolytes, and consequently results in the increased internal contact and charge-transfer resistance of the cells, which are responsible for the failure of the Li-S batteries under lean-ether-electrolyte conditions. We also demonstrate that by replacing the ether electrolytes with a sparingly solvating electrolyte, the electrochemical performance of the lean-electrolyte Li-S batteries could be markedly improved, which directs the future development of the high-energy Li-S batteries." @default.
• W3136234979 created "2021-03-29" @default.
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• W3136234979 date "2021-06-01" @default.
• W3136234979 modified "2023-10-16" @default.
• W3136234979 title "The Failure Mechanism of Lithium-Sulfur Batteries under Lean-Ether-Electrolyte Conditions" @default.
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• W3136234979 doi "https://doi.org/10.1016/j.ensm.2021.03.014" @default.
• W3136234979 hasPublicationYear "2021" @default.
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