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- W3136239676 abstract "Overcoming the limited light harvest and sluggish charge transfer efficiency has remained a long-standing challenge for the practical application of visible-light driven hydrogen evolution. In this work, a novel cobalt doped titanium nitride interlaced nanotube was synthesized through a facile hydrothermal approach and subsequent ammonia gas nitrification route. The optimized Ti0·75Co0·25N (molar ratio of Ti:Co:N = 0.75:0.25:1) catalyst delivered the highest hydrogen yield in visible-light-induced water splitting, which was almost 2 times higher than the pristine TiN did. Further structure characterizations have unraveled that the cobalt atoms were partially substituted the titanium atoms in crystallite lattice, generating a significant synergistic regulation on band structure and electronic state. As a result, the narrowed energy bandgap, improved charge carrier mobility and lowered over-potential contributed to the high electron-hole separation efficiency and smoothed interface charge transfer, yielding an enhanced photocatalytic activity. This work is a significant contribution to the design of efficient and stable visible light driven water splitting catalysts." @default.
- W3136239676 created "2021-03-29" @default.
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- W3136239676 date "2021-05-01" @default.
- W3136239676 modified "2023-10-01" @default.
- W3136239676 title "Tunable cobalt doping titanium nitride (Ti Co N) interlaced nanotubes enable an enhanced electronic synergy on visible-light driven hydrogen evolution" @default.
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- W3136239676 doi "https://doi.org/10.1016/j.ijhydene.2021.02.132" @default.
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