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- W3136246210 abstract "• Highly microporous amino-functionalized hyper-crosslinked resins are synthesized. • Aminated hyper-crosslinked resins show enhanced selective adsorption of CO 2. • Aminated hyper-crosslinked resins show 4 times increased indigo carmine adsorption. • Aminated resins show higher breakthrough adsorption of indigo carmine. New amino-functionalized vinylbenzyl chloride/divinylbenzene-based hyper-crosslinked resins (HCLRs) were synthesized with the objective of improving the HCLR polarity and affinity to carbon dioxide and polar dyes. The HCLRs chemical structure and textural properties were investigated and correlated to the adsorption performance of the modified (XDV-NH 2 ) and plain resin (XDV). The functionalization induced a reduction of the HCLR total porosity, while promoting the formation of a highly microporous structure with significant porosity narrower than 1 nm. Tested for CO 2 adsorption at 0 °C and 25 °C, despite a reduced total porosity, the amino-functionalized XDV-NH 2 resin showed up to 3 times increased adsorption capacity, higher CO 2 heat of adsorption and CO 2 /N 2 selectivity with respect to the pristine XDV. XDV-NH 2 also showed superior equilibrium and dynamic adsorption capacity of indigo carmine from solution with respect to XDV. These results demonstrate that the strategy proposed for the realization of amino-functionalized hyper-crosslinked resins is highly effective to obtain a microporous polymers with a significantly increased polar character and enhanced adsorption of CO 2 and polar dyes." @default.
- W3136246210 created "2021-03-29" @default.
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- W3136246210 date "2021-08-01" @default.
- W3136246210 modified "2023-10-02" @default.
- W3136246210 title "Amino-functionalized hyper-crosslinked resins for enhanced adsorption of carbon dioxide and polar dyes" @default.
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- W3136246210 doi "https://doi.org/10.1016/j.cej.2021.129463" @default.
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