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- W3136351593 abstract "Research on coordination polymers (CPs) using 2-deoxy-d-ribose derivatives as ligands has not been documented to the best of our knowledge. Herein, the new ligand L (1,3,4-trikisisoniacyl-2-deoxy-β-d-ribopyranose) was designed and synthesized from 2-deoxy-d-ribose, and four CPs {[MnL2Cl2]·4CH3OH}∞ (1), {[CoL2Cl2]·4CH3OH}∞ (2), {[NiL2Cl2]·4CH3OH}∞ (3) and {[CoL2Br2]·4CH3OH}∞ (4) were prepared using L as the bridging ligand. Single-crystal X-ray analyses showed that the above four CPs crystallize in the trigonal space group P3121 and have the same 2D grid structures with the same 1D meso-helices and the same 3D supramolecular architectures, and each metal center bonds with four pyridyl rings to form a Δ-propeller configuration in 1–4. The same space groups, structures, and chiral types of the propellers of 1–4 suggest that L is a powerful ligand in controlling the structures and chiralities of its metal complexes. Interestingly, 3 gave weaker emission in the solid state but much stronger emission in suspension, and 2–4 showed the ability to sense Fe3+ with LODs of 2.75, 0.12, and 0.87 μM and quenching constants of 1.07 × 104, 1.67 × 104, and 3.33 × 104 M–1, respectively, and high interference resistance, indicating their potential to be used as sensitive fluorescence sensors for detecting Fe3+. The different metal centers of 1–4 should be the main factors that make them distinct in fluorescent properties and probe functions due to the similarities in compositions and structures of the four CPs." @default.
- W3136351593 created "2021-03-29" @default.
- W3136351593 creator A5012537955 @default.
- W3136351593 creator A5058155763 @default.
- W3136351593 creator A5064026144 @default.
- W3136351593 creator A5073117227 @default.
- W3136351593 creator A5089600222 @default.
- W3136351593 date "2021-03-24" @default.
- W3136351593 modified "2023-10-16" @default.
- W3136351593 title "Chiral Coordination Polymers from a New 2-Deoxy-<scp>d</scp>-ribose Derivative Linker: Syntheses, Structures, and Fe<sup>3</sup><sup>+</sup> Fluorescent Probe Functions" @default.
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- W3136351593 doi "https://doi.org/10.1021/acs.cgd.0c01661" @default.
- W3136351593 hasPublicationYear "2021" @default.
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