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• W3136357887 endingPage "4771" @default.
• W3136357887 startingPage "4762" @default.
• W3136357887 abstract "Natural toxins are multifunctional, often ionizable organic compounds increasingly detected in the environment. Surprisingly little is known about their interactions with soil organic carbon, although sorption largely controls transport, bioavailability, and dissipation. For a set of 117 natural toxins from 36 compound classes the pH-dependent organic carbon–water distribution coefficient (Doc) was quantified using a soil column chromatography approach under changing conditions with regards to pH, ionic strength, and the major inorganic cation in solution. Natural toxins could be assigned to groups with either hydrophobic partitioning or specific interactions (complexation reactions, cation exchange) as dominating sorption mechanisms. The complex interplay of interactions in the sorption of natural toxins was equally influenced by sorbate, sorbent, and solution specific characteristics. High variability in sorption was particularly observed in the presence of Ca2+ resulting in Doc being enhanced by a factor of 10 when the pH was increased from 4.5 to 6. Sorbates following this trend contain either functional groups able to form ternary complexes via Ca2+ or aromatic moieties adjacent to protonated N presumably stabilizing cation exchange reactions. Although sorption was often stronger than predicted, investigated natural toxins were highly mobile under all considered conditions." @default.
• W3136357887 created "2021-03-29" @default.
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• W3136357887 creator A5042791363 @default.
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• W3136357887 date "2021-03-23" @default.
• W3136357887 modified "2023-10-11" @default.
• W3136357887 title "Disentangling Mechanisms in Natural Toxin Sorption to Soil Organic Carbon" @default.
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• W3136357887 doi "https://doi.org/10.1021/acs.est.0c06634" @default.
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• W3136357887 hasPublicationYear "2021" @default.
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