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- W3136381458 abstract "The thermodynamics of glasses and of the glass transition is reviewed phenomenologically. In view of its irreversible, kinetic nature, this transition cannot be described by equilibrium thermodynamics. The basic nonequilibrium concepts of order parameter and affinity are thus introduced to describe it and the properties of glasses, which cannot be represented in terms of only two state variables such as temperature and pressure. Calorimetric measurements on PolyVinylAcetate (PVAc) are in particular used to determine configurational heat capacities, enthalpies, and entropies and their variations when internal equilibrium is lost in the glass transition range. These variations can be accounted for with relaxation models, which can in addition clearly distinguish the entropy irreversibly produced at the glass transition from the variations of the configurational entropy of the glass-forming liquid." @default.
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- W3136381458 date "2021-02-01" @default.
- W3136381458 modified "2023-10-13" @default.
- W3136381458 title "Thermodynamics of Glasses" @default.
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- W3136381458 doi "https://doi.org/10.1002/9781118801017.ch3.2" @default.
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