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- W3136705313 abstract "A core–shell approach that utilizes a high-surface-area conducting core and an outer semiconductor shell is exploited here to prepare p-type dye-sensitized solar energy cells that operate with a minimal applied bias. Photocathodes were prepared by coating thin films of nanocrystalline indium tin oxide with a 0.8 nm Al2O3 seeding layer, followed by the chemical growth of nonstoichiometric strontium titanate. Films were annealed and sensitized with either a porphyrin chromophore or a chromophore–catalyst molecular assembly consisting of the porphyrin covalently tethered to the ruthenium complex. The sensitized photoelectrodes produced cathodic photocurrents of up to −315 μA/cm2 under simulated sunlight (AM1.5G, 100 mW/cm2) in aqueous media, pH 5. The photocurrent was increased by the addition of regenerative hole donors to the system, consistent with slow interfacial recombination kinetics, an important property of p-type dye-sensitized electrodes." @default.
- W3136705313 created "2021-03-29" @default.
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- W3136705313 date "2021-03-22" @default.
- W3136705313 modified "2023-09-26" @default.
- W3136705313 title "Dye-Sensitized Nonstoichiometric Strontium Titanate Core–Shell Photocathodes for Photoelectrosynthesis Applications" @default.
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- W3136705313 doi "https://doi.org/10.1021/acsami.1c00933" @default.
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