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• W3136759994 abstract "This paper describes the simple, highly reproducible, and robust synthesis of a new solid organic/inorganic electrolyte based on the ionic liquid (IL) 1-butyl-3-(carboxyundecyl)imidazolium bis(trifluoromethylsulfonyl)imide tethered to zirconia nanoparticles (15–25 nm) by coordination and named ZrO2@IL. The IL monolayer formation, ensured by two-dimensional solid-state NMR, at the nanoparticles’ surface considerably reduces both the IL’s consumption and the IL amount at the ZrO2 surface compared to the IL-based hybrid electrolytes reported in the literature. After LiTFSI, used as a lithium source, content optimization (26 wt %), the hybrid exhibits unprecedented stable conductivity passing from 0.6 × 10–4 S.cm–1 to 0.15 × 10–4 S.cm–1, respectively, from 85 °C to room temperature (25 °C). Unlike silica which is commonly adopted for this type of hybrid material, zirconia makes it possible to produce more impact-resistant pellets that are easier to compact, thus being favorable for accurate conductivity studies and battery development by electrode/composite/solid electrolyte layer stacking. The ZrO2@IL/LiTFSI solid hybrid electrolyte’s thermal stability (up to 300 °C) and performance make this electrolyte suitable for lithium conduction in all-solid-state batteries." @default.
• W3136759994 created "2021-03-29" @default.
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• W3136759994 date "2021-03-24" @default.
• W3136759994 modified "2023-10-16" @default.
• W3136759994 title "Hybrid Electrolytes Based on Optimized Ionic Liquid Quantity Tethered on ZrO₂ Nanoparticles for Solid-State Lithium-Ion Conduction" @default.
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• W3136759994 doi "https://doi.org/10.1021/acsami.0c22422" @default.
• W3136759994 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33760585" @default.
• W3136759994 hasPublicationYear "2021" @default.
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