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• W3137109279 startingPage "3210" @default.
• W3137109279 abstract "Selective catalytic reduction of NOx with NH3 (NH3–SCR) in Cu-SSZ-13 has been proposed to have a unique homogeneous-like mechanism governed by the spatial proximity of mobile Cu ions. Among factors that determine the proximity, the effect of ion density on the SCR reaction is well established; however, it has not been verified how the different mobility of the Cu ion influences the SCR reaction. Herein, we try to reveal the mobility-dependent SCR reaction by controlling the Cu species with different ion mobilities in Cu-SSZ-13. Since the reaction kinetics is governed by the diffusion of Cu ions, the Cu ion mobility determines the reactivity of the Cu-SSZ-13. In terms of this correlation, enhanced ion mobility leads to improved NH3–SCR activity. These findings help understand the behavior of Cu ions in Cu-SSZ-13 under a catalytic reaction and provide insights to design rational catalysts by tuning the ion mobility." @default.
• W3137109279 created "2021-03-29" @default.
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• W3137109279 creator A5072531739 @default.
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• W3137109279 date "2021-03-24" @default.
• W3137109279 modified "2023-10-07" @default.
• W3137109279 title "Mobility of Cu Ions in Cu-SSZ-13 Determines the Reactivity of Selective Catalytic Reduction of NO_<i>x</i> with NH₃" @default.
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• W3137109279 doi "https://doi.org/10.1021/acs.jpclett.1c00181" @default.
• W3137109279 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33761261" @default.
• W3137109279 hasPublicationYear "2021" @default.
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