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- W3137185853 abstract "A highly enantioselective three-component reaction of ynamides with carboxylic acids and 2,2′-diester aziridines has been realized by using a chiral N,N′-dioxide/Ho(OTf)3 complex as a Lewis acid catalyst. The process includes the formation of an α-acyloxyenamide intermediate through the addition of carboxylic acids to ynamides and the following enantioselective nucleophilic addition to in-situ-generated azomethine ylides induced by the chiral catalyst. A range of amino acyloxyenamides are delivered in moderate to good yields with good ee values. In addition, a possible catalytic cycle with a transition model is proposed to elucidate the reaction mechanism." @default.
- W3137185853 created "2021-03-29" @default.
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- W3137185853 date "2021-03-26" @default.
- W3137185853 modified "2023-10-17" @default.
- W3137185853 title "Catalytic Asymmetric Hydroacyloxylation/Ring-Opening Reaction of Ynamides, Acids, and Aziridines" @default.
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- W3137185853 doi "https://doi.org/10.1021/acs.orglett.1c00631" @default.
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