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- W3137521122 endingPage "4404" @default.
- W3137521122 startingPage "4397" @default.
- W3137521122 abstract "Hydrogen peroxide is a dynamic signaling molecule in biological systems. We report herein a versatile double emulsion sensor that can detect femtomolar quantities of aqueous hydrogen peroxide. The mechanism responsible for this sensitivity is a peroxide induced change in double emulsion structure, which results in a modified directional emission from dyes dissolved in the high index organic phase. The morphology (structure) of the double emulsion is controlled via interfacial tensions and a methyltrioxorhenium catalyzed sulfide oxidation results in an enhancement of the surfactant effectiveness. The incipient polar sulfoxide induced decrease of the interfacial tension at the organic-water (O–W) interface results in an increased interfacial area between the organic phase and water and a diminished emission perpendicular to the supporting substrate. The modularity of our sensory system is demonstrated through cascade catalysis between methyltrioxorhenium and oxidase enzymes, with the latter producing hydrogen peroxide as a byproduct to enable for the selective and sensitive detection of molecular and ionic enzymatic substrates." @default.
- W3137521122 created "2021-03-29" @default.
- W3137521122 creator A5040213713 @default.
- W3137521122 creator A5045135784 @default.
- W3137521122 date "2021-03-16" @default.
- W3137521122 modified "2023-10-11" @default.
- W3137521122 title "Trace Detection of Hydrogen Peroxide via Dynamic Double Emulsions" @default.
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- W3137521122 doi "https://doi.org/10.1021/jacs.1c00683" @default.
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- W3137521122 hasPublicationYear "2021" @default.
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