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- W3137639741 abstract "Abstract Core–shell nanocomposites with a catalytic metal-organic framework (MOF) shell are more effective and stable than bare MOF. We have successfully designed an effective heterogeneous catalyst for the synthesis of benzimidazole by integrating acidic catalytic activity, and promoted the aerobic oxidation and magnetic recyclability of core–shell nanocomposite Fe 3 O 4 @SiO 2 @UiO-66. The Fe 3 O 4 @SiO 2 core is encapsulated by the in situ- grown UiO-66 shell, and the UiO-66 shell retains the porous structure and crystallinity of UiO-66 with abundant exposed Lewis acid sites. It shows high catalytic ability for the synthesis of various benzimidazoles through the acid-catalyzed condensation and aerobic oxidation with in situ oxygen. The Fe 3 O 4 @SiO 2 core provides magnetic recyclability of Fe 3 O 4 @SiO 2 @UiO-66, and maintains high catalytic ability and stability over six cycles." @default.
- W3137639741 created "2021-03-29" @default.
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- W3137639741 date "2021-04-09" @default.
- W3137639741 modified "2023-09-25" @default.
- W3137639741 title "Novel core–shell nanocomposite as an effective heterogeneous catalyst for the synthesis of benzimidazoles" @default.
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- W3137639741 doi "https://doi.org/10.1088/1361-6528/abef2f" @default.
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