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• W3137799265 endingPage "108798" @default.
• W3137799265 startingPage "108798" @default.
• W3137799265 abstract "Despite the great progress on the development of zinc ion batteries (ZIBs) in recent years, the issue of zinc corrosion in aqueous media and the associated dendrite growth of the electrode remains a major challenge for achieving high-performance anode materials with long-term stability. Herein, we report a facile, yet, effective interfacial optimization of zinc (Zn) anode using a nanofluidic channel (NC) layer made up of Poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT:PSS) decorated graphene sheets (GSs) produced by electrochemical exfoliation. The NCs effectively modulated the Zn ion distribution density, inhibited dendrite growth, and restrained other side reactions due to its tunable channel size and the surface functional groups. Moreover, the extra conductive polymer (PEDOT:PSS) on the NC layer curbed the polarization problem by enhancing the electric field on the Zn anode. As a result, PEDOT:PSS/GS@Zn anode demonstrated prolonged cycling stability for 8000 cycles with substantial improvements in specific discharge capacity due to the enhanced electron transit efficiency. In summary, our work proposes a scalable technological approach to fabricate dendrite-free Zn anodes and provides a universal inspiration to restrain dendrite formation during the ion electroplating processes. • PEDOT:PSS modified GSs are mass produced by electrochemical exfoliation method. • NC layer is constructed to guide ion distribution density for Zinc anode. • NC layer effectively inhibits the detrimental dendrite growth and side reactions. • PEDOT:PSS/GS@Zn anode demonstrates excellent cycling stability for 8000 cycles." @default.
• W3137799265 created "2021-03-29" @default.
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• W3137799265 date "2021-06-01" @default.
• W3137799265 modified "2023-10-15" @default.
• W3137799265 title "Constructing PEDOT:PSS/Graphene sheet nanofluidic channels to achieve dendrite-free Zn anode" @default.
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• W3137799265 doi "https://doi.org/10.1016/j.compositesb.2021.108798" @default.
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