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• W3137971312 abstract "Two-dimensional (2D) material-based membranes hold great promise in wastewater treatment. However, it remains challenging to achieve highly efficient and precise small molecule/ion separation with pure 2D material-fabricated lamellar membranes. In this work, laminated graphene oxide (GO)–cellulose nanocrystal (CNC) hybrid membranes (GO/CNC) were fabricated by taking advantages of the unique structures and synergistic effects generated from these two materials. The characterization results in physiochemical properties, and the structure of the as-synthesized hybrid membranes displayed enhanced membrane surface hydrophilicity, enhanced crumpling surface structure, and slightly enlarged interlayer-spacing with the incorporation of CNCs. Water permeability increases by two to four times with the addition of different CNC weight ratios in comparison to a pristine GO membrane. The optimal GO/CNC membrane achieved efficient rejection toward three typical antibiotics at 74.8, 90.9, and 97.2% for sulfamethoxazole (SMX), levofloxacin (Levo), and norfloxacin (Nor), respectively, while allowing a high passage of desirable nutrients such as NO3– and H2PO4–. It was found that SMX removal is primarily governed by electrostatic repulsion, while adsorption plays a crucial role in removing Levo and Nor. Moreover, the density functional theory calculations confirmed the increased antibiotic removal in the presence of an organic foulant, humic acid. Such a 2D material-based hybrid membrane offers a new strategy to develop fit-for purpose membranes for resource recovery and water separation." @default.
• W3137971312 created "2021-03-29" @default.
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• W3137971312 date "2021-03-19" @default.
• W3137971312 modified "2023-10-06" @default.
• W3137971312 title "Incorporation of Cellulose Nanocrystals into Graphene Oxide Membranes for Efficient Antibiotic Removal at High Nutrient Recovery" @default.
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• W3137971312 doi "https://doi.org/10.1021/acsami.0c20652" @default.
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• W3137971312 hasPublicationYear "2021" @default.
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