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• W3138200430 abstract "This paper describes a new method for the transannular functionalization of the γ-C-H bonds in alicyclic amines to install C(sp3 )-halogen, oxygen, nitrogen, boron, and sulfur bonds. The key challenge for this transformation is controlling the relative rate of Cγ -H versus Cα -H functionalization. We demonstrate that this selectivity can be achieved by pre-complexation of the substrate with Pd prior to the addition of oxidant. This approach enables the use of diverse oxidants that ultimately install various heteroatom functional groups at the γ-position with high site- and diastereoselectivity." @default.
• W3138200430 created "2021-03-29" @default.
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• W3138200430 date "2021-04-08" @default.
• W3138200430 modified "2023-09-27" @default.
• W3138200430 title "Palladium‐Mediated C _γ −H Functionalization of Alicyclic Amines" @default.
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• W3138200430 doi "https://doi.org/10.1002/anie.202101782" @default.
• W3138200430 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8102420" @default.
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