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• W3139486522 abstract "The use of stoichiometric organoborane reductants in organic synthesis is well established. Here these reagents have been rendered catalytic through an isodesmic B-O/B-H transborylation applied in the borane-catalyzed, chemoselective alkene reduction and formal hydrofunctionalization of enones. The reaction was found to proceed by a 1,4-hydroboration of the enone and B-O/B-H transborylation with HBpin, enabling catalyst turnover. Single-turnover and isotopic labeling experiments supported the proposed mechanism of catalysis with 1,4-hydroboration and B-O/B-H transborylation as key steps." @default.
• W3139486522 created "2021-03-29" @default.
• W3139486522 creator A5030459737 @default.
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• W3139486522 date "2021-03-16" @default.
• W3139486522 modified "2023-09-27" @default.
• W3139486522 title "Borane-Catalyzed, Chemoselective Reduction and Hydrofunctionalization of Enones Enabled by B–O Transborylation" @default.
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• W3139486522 doi "https://doi.org/10.1021/acs.orglett.1c00446" @default.
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