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- W3140121911 abstract "Reversible hydrogen absorption/desorption, the very fundamental property of metal hydrides (MHs), can be utilized to innovate the water splitting process. Spontaneous hydrogen absorption by a MH electrode shifts the water reduction potential to 0.3 V above the reversible hydrogen electrode. Then, the absorbed hydrogen can be released to give H2 by thermal dehydrogenation at mild temperature below 70 °C by utilizing low grade heat. The MH mediated water splitting combines the electrochemical hydrogen absorption in Ni-MH batteries and the thermal dehydrogenation in gas phase hydrogen storage, which significantly reduces the electrical energy consumption for water splitting up to 25 kJ (mol H2)−1 compared to an ideal hydrogen evolution catalyst and also automatically leads to decoupled H2/O2 generation. The advantages and mechanisms of the MH mediated water splitting are demonstrated by MH electrodes with surface Pd coating." @default.
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- W3140121911 date "2021-07-01" @default.
- W3140121911 modified "2023-10-18" @default.
- W3140121911 title "Metal hydride mediated water splitting: Electrical energy saving and decoupled H2/O2 generation" @default.
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- W3140121911 doi "https://doi.org/10.1016/j.mattod.2021.02.019" @default.
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