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- W31403463 abstract "Publisher Summary This chapter presents experimental results which appear to correlate internal conversion efficiency with a macroscopic parameter representing the intermolecular coupling strength. This has been established by investigating the temperature dependence of the solute fluorescence intensity of degassed organic liquid scintillator solutions from 20°–240°C. The temperature variation found for n e under high energy excitation therefore reflects that of n eo , the internal conversion efficiency. Relative values of n e at room temperature for six solutes in a common solvent (o-xylene) are found in the range 0.36–1.00. The intrinsic solute fluorescence efficiencies have been taken into account in determining these relative n e values. The values are normalized so that n e (20°C) for the o-xylene system is unity. The most efficient scintillator solutes are not only those with high intrinsic fluorescence efficiencies, but are also characterized by a large “trapping” efficiency with respect to the solvent. One is thus led to consider the parameter n e as a product of two factors, n e = n eo K. The parameter K is found to be temperature-invariant for all systems tested. The factor n eo (under UV solvent excitation) is assumed constant since the extinction coefficient, a related parameter, is not known to be temperature dependent. However, the major factor affecting internal conversion efficiency is the intermolecular coupling strength." @default.
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- W31403463 date "1971-01-01" @default.
- W31403463 modified "2023-09-23" @default.
- W31403463 title "POPULATION OF TRANSFER STATES IN LIQUID SCINTILLATORS VIA A TEMPERATURE STUDY" @default.
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- W31403463 doi "https://doi.org/10.1016/b978-0-12-356250-0.50023-3" @default.
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