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- W3140509301 abstract "Developing an efficient and simple heterogeneous catalytic system for CO2 conversion into formic acid (FA) is a vibrant research area because FA is recognized as a liquid organic hydrogen carrier. On the basis of our previous work on unsupported nanoporous palladium-catalyzed hydrogenation proceeding through a Pd-hydride intermediate, we report herein four types of PdNPore catalysts for the CO2 hydrogenation. The PdNPore-1 catalyst exhibited high catalytic activity for CO2 hydrogenation into formate and obtained a yield of 86 % at 80 °C under H2 (1.0 MPa) and CO2 (1.5 MPa) with 1,8-diazabicyclo[5.4.0]undec-7-ene (DBU) as a base in acetonitrile. Moreover, the catalyst was easily recovered and reused without any loss of catalytic activity. Sodium bicarbonate could also be hydrogenated using the PdNPore-1 catalyst." @default.
- W3140509301 created "2021-04-13" @default.
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- W3140509301 date "2021-04-26" @default.
- W3140509301 modified "2023-10-16" @default.
- W3140509301 title "Unsupported Nanoporous Palladium Catalyst for Highly Selective Hydrogenation of Carbon Dioxide and Sodium Bicarbonate into Formate" @default.
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- W3140509301 doi "https://doi.org/10.1002/cctc.202100148" @default.
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