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- W3140654086 endingPage "13912" @default.
- W3140654086 startingPage "13906" @default.
- W3140654086 abstract "Abstract A series of rhenium complexes bearing a pyridine‐based PNP‐type pincer ligand are synthesized from rhenium phosphine complexes as precursors. A dinitrogen‐bridged dirhenium complex bearing the PNP‐type pincer ligands catalytically converts dinitrogen into ammonia during the reaction with KC 8 as a reductant and [HPCy 3 ]BAr F 4 (Cy=cyclohexyl, Ar F =3,5‐(CF 3 ) 2 C 6 H 3 ) as a proton source at −78 °C to afford 8.4 equiv of ammonia based on the rhenium atom of the catalyst. The rhenium‐dinitrogen complex also catalyzes silylation of dinitrogen in the reaction with KC 8 as a reductant and Me 3 SiCl as a silylating reagent under ambient reaction conditions to afford 11.7 equiv of tris(trimethylsilyl)amine based on the rhenium atom of the catalyst. These results demonstrate the first successful example of catalytic nitrogen fixation under mild reaction conditions using rhenium‐dinitrogen complexes as catalysts." @default.
- W3140654086 created "2021-04-13" @default.
- W3140654086 creator A5008539128 @default.
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- W3140654086 creator A5053204418 @default.
- W3140654086 creator A5067878871 @default.
- W3140654086 creator A5069936893 @default.
- W3140654086 date "2021-05-10" @default.
- W3140654086 modified "2023-09-30" @default.
- W3140654086 title "Ammonia Formation Catalyzed by a Dinitrogen‐Bridged Dirhenium Complex Bearing PNP‐Pincer Ligands under Mild Reaction Conditions**" @default.
- W3140654086 cites W1915409416 @default.
- W3140654086 cites W1992590478 @default.
- W3140654086 cites W1992825078 @default.
- W3140654086 cites W1999867559 @default.
- W3140654086 cites W2003431221 @default.
- W3140654086 cites W2004038548 @default.
- W3140654086 cites W2030901776 @default.
- W3140654086 cites W2037335872 @default.
- W3140654086 cites W2040939995 @default.
- W3140654086 cites W2043772300 @default.
- W3140654086 cites W2048110396 @default.
- W3140654086 cites W2052873679 @default.
- W3140654086 cites W2067905788 @default.
- W3140654086 cites W2087280723 @default.
- W3140654086 cites W2090749185 @default.
- W3140654086 cites W2116880127 @default.
- W3140654086 cites W2133766418 @default.
- W3140654086 cites W2145959116 @default.
- W3140654086 cites W2147845885 @default.
- W3140654086 cites W2155324577 @default.
- W3140654086 cites W2158012127 @default.
- W3140654086 cites W2165882368 @default.
- W3140654086 cites W2295535048 @default.
- W3140654086 cites W2296527166 @default.
- W3140654086 cites W2314603695 @default.
- W3140654086 cites W2315707420 @default.
- W3140654086 cites W2317239842 @default.
- W3140654086 cites W2320459612 @default.
- W3140654086 cites W2321353110 @default.
- W3140654086 cites W2331988401 @default.
- W3140654086 cites W2333815467 @default.
- W3140654086 cites W2418943070 @default.
- W3140654086 cites W2499262475 @default.
- W3140654086 cites W2512854279 @default.
- W3140654086 cites W2529904852 @default.
- W3140654086 cites W2577341763 @default.
- W3140654086 cites W2588590309 @default.
- W3140654086 cites W2603128986 @default.
- W3140654086 cites W2604147093 @default.
- W3140654086 cites W2604447493 @default.
- W3140654086 cites W2612972784 @default.
- W3140654086 cites W2626189122 @default.
- W3140654086 cites W2626460967 @default.
- W3140654086 cites W2725199309 @default.
- W3140654086 cites W2736771995 @default.
- W3140654086 cites W2765274473 @default.
- W3140654086 cites W2768395972 @default.
- W3140654086 cites W2784197008 @default.
- W3140654086 cites W2785552471 @default.
- W3140654086 cites W2790386365 @default.
- W3140654086 cites W2794686155 @default.
- W3140654086 cites W2797768937 @default.
- W3140654086 cites W2801609803 @default.
- W3140654086 cites W2805155466 @default.
- W3140654086 cites W2810580056 @default.
- W3140654086 cites W2828255577 @default.
- W3140654086 cites W2883029073 @default.
- W3140654086 cites W2887758551 @default.
- W3140654086 cites W2893689217 @default.
- W3140654086 cites W2901406848 @default.
- W3140654086 cites W2911746849 @default.
- W3140654086 cites W2914921060 @default.
- W3140654086 cites W2920050533 @default.
- W3140654086 cites W2927123968 @default.
- W3140654086 cites W2941357953 @default.
- W3140654086 cites W2945750681 @default.
- W3140654086 cites W2949855829 @default.
- W3140654086 cites W2955117213 @default.
- W3140654086 cites W2967111369 @default.
- W3140654086 cites W2988744248 @default.
- W3140654086 cites W2990527982 @default.
- W3140654086 cites W2993170768 @default.
- W3140654086 cites W2996023859 @default.
- W3140654086 cites W2999927570 @default.
- W3140654086 cites W3000410519 @default.
- W3140654086 cites W3006712405 @default.
- W3140654086 cites W3008880133 @default.
- W3140654086 cites W3022216159 @default.
- W3140654086 cites W3023120551 @default.
- W3140654086 cites W3030209662 @default.
- W3140654086 cites W3047035729 @default.
- W3140654086 cites W3086122596 @default.
- W3140654086 cites W3110956173 @default.
- W3140654086 cites W3119728328 @default.
- W3140654086 cites W3127597104 @default.
- W3140654086 cites W3133623367 @default.
- W3140654086 cites W4230208330 @default.