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• W3141801914 abstract "Nanostructured palladium catalysts are used industrially for selective alkyne hydrogenation reactions. However, structural changes can lead to a loss of performance. In this study, we show the evolution of the atomic structure of monodispersed Pd nanoclusters undergoing a vapour-phase 1-pentyne hydrogenation reaction. A specific structural transformation, from amorphous to highly symmetrical structures, is observed at the atomic level with aberration-corrected scanning transmission electron microscopy (AC-STEM). This surprising behaviour which occurs concurrently with the alkyne hydrogenation reaction, is clearly size-dependent. The results provide new understanding of the long-term stability of commercial heterogeneous catalysts." @default.
• W3141801914 created "2021-04-13" @default.
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• W3141801914 date "2021-05-01" @default.
• W3141801914 modified "2023-09-26" @default.
• W3141801914 title "From amorphous to ordered: Structural transformation of Pd nanoclusters in 1-pentyne hydrogenation reactions" @default.
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• W3141801914 doi "https://doi.org/10.1016/j.jcat.2021.03.019" @default.
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