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- W3142039956 abstract "To minimize the harmful environmental effects from CO2 emissions, technologies for carbon capture and CO2 recycling are needed to sustainably produce value-added chemicals and supplement photosynthetic carbon cycle. In this chapter, the development of heterogeneous catalysts and processes for the direct CO2 hydrogenation to alcohols are summarized from past to present, with special emphasis on thermodynamics considerations, catalyst designs, mechanistic aspects, and recent advances. We first introduce a more selective and technologically mature route for alcohol synthesis from CO2 hydrogenation to methanol, a key chemical for oil-independent economy (methanol economy). The major challenge, apart from high energy cost for CO2 capture and H2 production, remains the true understanding of the active sites and reaction mechanism. Afterward, we discuss a more challenging synthesis of higher alcohols (C2+) that are more desirable as an energy vector and more compatible with the current fuel infrastructure. Major challenges continue to be the limited chain growth toward higher alcohols and the catalyst design to optimize both CO2 reduction and chain propagation. Finally, CO2 hydrogenation to alcohols still requires some improvements in catalyst and process design to achieve a commercially attractive catalytic performance." @default.
- W3142039956 created "2021-04-13" @default.
- W3142039956 creator A5018595294 @default.
- W3142039956 creator A5024785758 @default.
- W3142039956 date "2021-03-08" @default.
- W3142039956 modified "2023-10-16" @default.
- W3142039956 title "Heterogeneously Catalyzed CO2 Hydrogenation to Alcohols" @default.
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