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• W3144178872 abstract "Efficient removal of uranium (U) from aqueous solutions is crucial for ecological safety. Functionalized magnetic nanoparticles provide a promising strategy for radionuclide recovery and separation. However, designing and synthesizing magnetic adsorbents with high sorption capacity and selectivity, accompanied by excellent stability and reusability, remain a challenge. In this work, novel amidoxime-functionalized flower-like magnetic Fe3O4@TiO2 core-shell microspheres are designed and synthesized to efficiently remove U(VI) from aqueous solutions and actual seawater. The magnetic Fe3O4 core facilitates easy separation by an external magnetic field, and flower-like TiO2 nanosheets provide abundant specific surface areas and functionalization sites. The grafted amidoxime (AO) groups could function as a claw for catching uranium. The maximum adsorption capacity on U(VI) of the designed nanospheres reaches 313.6 mg·g-1 at pH 6.0, and the adsorption efficiency is maintained at 97% after 10 cycles. In addition, the excellent selectivity of the magnetic recyclable AO-functioning Fe3O4@TiO2 microspheres endows the potential of uranium extraction from seawater. The designed material provides an effective and applicable diagram for radioactive element elimination and enrichment." @default.
• W3144178872 created "2021-04-13" @default.
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• W3144178872 date "2021-04-06" @default.
• W3144178872 modified "2023-10-16" @default.
• W3144178872 title "An Efficient Uranium Adsorption Magnetic Platform Based on Amidoxime-Functionalized Flower-like Fe₃O₄@TiO₂ Core–Shell Microspheres" @default.
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• W3144178872 doi "https://doi.org/10.1021/acsami.1c00556" @default.
• W3144178872 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33821605" @default.
• W3144178872 hasPublicationYear "2021" @default.
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