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- W3144516766 abstract "Bimetallic Au/Pd nanoparticles were prepared and used to catalyze oxidation of alcohols in the poly(ethylene glycol) (PEG)/CO2 biphasic system using O2 as the oxidant without adding any base.The catalytic activity of Au/Pd bimetal with different mole ratios was studied using benzyl alcohol as the substrate.It was found that bimetallic Au/Pd nanoparticles with Au:Pd=1:3.5 had higher catalytic activity than monometallic Au,Pd and the bimetallic Au/Pd nanoparticles with other molar ratios.The effect of CO2 pressure on the oxidation of benzyl alcohol and 1-phenylethanol in PEG/CO2 was investigated.It was demonstrated that CO2 pressure could be used to tune the conversion and selectivity of the reactions effectively.α,β-Unsaturated alcohols were also studied and found to be more reactive than benzyl alcohol and 1-phenylethanol.Recycling experiments showed that the Au/Pd/PEG/CO2 catalytic system could be recycled at least four times without reducing the activity.In addition,the catalytic system is clean and the products can be separated easily." @default.
- W3144516766 created "2021-04-13" @default.
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- W3144516766 date "2010-01-01" @default.
- W3144516766 modified "2023-10-08" @default.
- W3144516766 title "Bimetallic Au/Pd catalyzed aerobic oxidation of alcohols in the poly(ethylene glycol)/CO_2 system" @default.
- W3144516766 hasPublicationYear "2010" @default.
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