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- W3144857891 abstract "Abstract Anthrathiadiazole is a key synthon for the construction of large azaacenes, however, the attachment of different substituents onto the skeleton of anthrathiadiazole is difficult but highly desirable because it could be easy to enrich the structures of azaacenes. Here, it is demonstrated that anthrathiadiazole derivatives with −Br, −CN, and −OCH 3 groups could be easily constructed through a simple [4+2] cycloaddition reaction between a,a,a’,a’ ‐tetrabromo ‐o ‐xylenes derivatives and benzo[c][1,2,5]thiadiazole‐4,7‐dione. The structures of the as‐prepared compounds with different substituents were carefully characterized. Moreover, the basic physical properties of the as‐prepared anthrathiadiazole derivatives were fully investigated, where the cyano‐substituted derivative (BTH ‐ CN) has the highest stability and the methoxy‐substituted derivative ( BTH ‐ OCH 3 ) is easy to be oxidized. Moreover, the two‐photon absorption (TPA) characteristics of different anthrathiadiazoles are also studied by using the femtosecond Z‐scan technique. The results show that the fused anthrathiadiazole skeletons possess large TPA cross‐section values δ 2 in the range of 3000–5000 GM, where the nature, position and strength of the substituted groups have strong effect on these values." @default.
- W3144857891 created "2021-04-13" @default.
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- W3144857891 date "2021-06-21" @default.
- W3144857891 modified "2023-10-18" @default.
- W3144857891 title "Anthrathiadiazole Derivatives: Synthesis, Physical Properties and Two‐photon Absorption" @default.
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- W3144857891 doi "https://doi.org/10.1002/chem.202100307" @default.
- W3144857891 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33780036" @default.
- W3144857891 hasPublicationYear "2021" @default.
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