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• W3146099964 abstract "Chemistry at interface, i.e., at the junction between two immiscible bulk media is remarkably different from either of the bulk phases. This is primarily due to an anisotropic environment at interface where reactants behave differently than they do in isotropic bulk media. Interface-selective spectroscopy can provide valuable insight into such interface specific phenomena at the molecular level. Presently, vibrational sum frequency generation (VSFG) is the best suited spectroscopic technique to unravel interfacial molecular properties, especially for the “soft interface” such as liquid surface where linear optical spectroscopy and particle scattering based techniques cannot be applied either due to the lack of interface-selectivity or due to requirement of stringent experimental conditions. VSFG is inherently interface-selective and probes molecules by their vibrational transitions, revealing site-specific molecular properties. This Chapter provides a brief description of the theory of VSFG followed by the origin of its interface-selectivity and detection of VSFG signal by the conventional (classical-VSFG) and heterodyne-detection (HD-VSFG) methods. Unlike classical-VSFG, HD-VSFG records unambiguous absorption spectra and absolute orientation of interfacial molecules. Finally, we discuss the application of narrowband classical-VSFG and broadband HD-VSFG techniques to aqueous interfaces of biological and environmental relevance. Specifically, the surface properties of ions, molecules, lipids, pollutants, and the associated perturbation of H-bonding and orientation of interfacial water." @default.
• W3146099964 created "2021-04-13" @default.
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• W3146099964 date "2021-01-01" @default.
• W3146099964 modified "2023-09-26" @default.
• W3146099964 title "Classical- and Heterodyne-Detected Vibrational Sum Frequency Generation (VSFG) Spectroscopy and Its Application to Soft Interfaces" @default.
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• W3146099964 doi "https://doi.org/10.1007/978-981-33-6084-6_4" @default.
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