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• W3147142416 abstract "Abstract Atomically dispersed Fe−N−C electrocatalysts have displayed excellent catalytic performances towards the oxygen reduction reaction (ORR), while the identification of the genuine active sites remains a challenge. Herein, we report a Fe−N−C electrocatalyst of FeSA/HNPC featuring single‐atomic FeN 4 sites on hierarchically N‐doped porous carbon (HNPC), which shows a very competitive ORR activity in alkaline solution even at a low electrocatalyst loading of 0.2 mg cm −2 on the working electrode. A comparison of energy barriers in ORR reveals that the single‐atomic FeN 4 active sites in FeSA/HNPC existing in the form of pyrrole‐N 4 −Fe is more favorable than that of pyridine‐N 4 −Fe for the enhanced ORR activity. Understanding the nature of FeN 4 active sites will greatly benefit the design of Fe−N−C electrocatalysts with highly effective ORR performances." @default.
• W3147142416 created "2021-04-13" @default.
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• W3147142416 date "2021-05-10" @default.
• W3147142416 modified "2023-10-17" @default.
• W3147142416 title "A Highly Efficient Fe−N−C Electrocatalyst with Atomically Dispersed FeN ₄ Sites for the Oxygen Reduction Reaction" @default.
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• W3147142416 doi "https://doi.org/10.1002/cctc.202100132" @default.
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