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- W3147890229 abstract "Impulsive orientation of symmetric-top molecules excited by two-color femtosecond pulses is considered. In addition to the well-known transient orientation appearing immediately after the pulse and then reemerging periodically due to quantum revivals, we report the phenomenon of field-free long-lasting orientation. Long-lasting means that the time averaged orientation remains non-zero until destroyed by other physical effects, e.g., intermolecular collisions. The effect is caused by the combined action of the field-polarizability and field-hyperpolarizability interactions. The dependence of degree of long-lasting orientation on temperature and pulse parameters is considered. The effect can be measured by means of second (or higher-order) harmonic generation, and may be used to control the deflection of molecules traveling through inhomogeneous electrostatic fields." @default.
- W3147890229 created "2021-04-13" @default.
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- W3147890229 date "2021-07-16" @default.
- W3147890229 modified "2023-09-23" @default.
- W3147890229 title "Long-Lasting Orientation of Symmetric-Top Molecules Excited by Two-Color Femtosecond Pulses" @default.
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- W3147890229 doi "https://doi.org/10.3389/fphy.2021.689635" @default.
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