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- W3148471444 abstract "Abstract The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behaviour, here we describe a system in which the structural disorder results in long-range antiferromagnetic order due to local symmetry breaking. Nd 2 ScNbO 7 is shown to have a dispersionless gapped excitation observed in other neodymium pyrochlores below T N = 0.37 K through polarized and inelastic neutron scattering. However the dispersing spin waves are not observed. This excited mode is shown to occur in only 14(2)% of the neodymium ions through spectroscopy and is consistent with total scattering measurements as well as the magnitude of the dynamic moment 0.26(2) μ B . The remaining magnetic species order completely into the all-in all-out Ising antiferromagnetic structure. This can be seen as a result of local symmetry breaking due disordered Sc +3 and Nb +5 ions about the A -site. From this work, it has been established that B -site disorder restores the dipole-like behaviour of the Nd +3 ions compared to the Nd 2 B 2 O 7 parent series." @default.
- W3148471444 created "2021-04-13" @default.
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- W3148471444 date "2021-05-14" @default.
- W3148471444 modified "2023-09-30" @default.
- W3148471444 title "Magnetic ordering in the Ising antiferromagnetic pyrochlore Nd<sub>2</sub>ScNbO<sub>7</sub>" @default.
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- W3148471444 doi "https://doi.org/10.1088/1361-648x/abf594" @default.
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