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- W3148665878 abstract "Cu/SiO2 catalysts prepared by different methods have been investigated focusing on the influence of Cu+on the catalytic performance.The composition,structure and copper valence state were characterized by means of BET,XRD,XPS,FTIR,N2O-titration.It was found that the Cu/SiO2 prepared by ammoniaevaporation（AE） method had much higher TOF value than that prepared by wetness-impregnation（WI）with the same THF selectivity.The higher TOF value was attributed to the coexistence of Cu+ and Cu0species in the activated AE-Cu/SiO2.while only Cu° species existing in the activated Wl-Cu/SiO2.Researches suggest that Cu+ can adsorb and polarize the C=0 bond of DMM.It is concluded that Cu°could be the main active site and the synergistic effect between Cu0 and Cu+ could contribute to hydrogenation of DMM to THF." @default.
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- W3148665878 date "2015-01-01" @default.
- W3148665878 modified "2023-09-28" @default.
- W3148665878 title "Selective hydrogenation of dimethyl maleate to tetrahydrofuran over Cu/SiO2 catalyst：Effect of Cu^＋ on the catalytic performance" @default.
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