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• W3150596379 endingPage "138282" @default.
• W3150596379 startingPage "138282" @default.
• W3150596379 abstract "The commercialization of lithium sulfur battery is greatly impeded by the severe capacity decay induced by polysulfides shuttle during charge/discharge process. Herein, we propose a composite carbon material with Co-N doping and high conductivity for polysulfides barrier layer. ZIF67 and high conductivity Ketjen Black(KB) are combined by a facile water solution reaction at room temperature at first, afterwords the as-prepared ZIF67/KB precursor is calcined in nitrogen atmosphere to obtain a novel Co-N/KB nano structure. The Co-N/KB hybrid is then coated on the commercial PE separator to improve electrochemical properties of Li-S battery. The Co-N/KB coating layer apparently promote the redox kinetics and show chemisorption ability toward polysulfides. Furthermore, the coating layer with high conductivity can also be used as a second current collector to promote the electronic transmission, which will increase the use ratio of active substances and improve the cycle retention. By the use of Co-N/KB modified separator, the initial discharge capacity of sulfur cathode with a sulfur areal loading of 3 mg cm−2 reaches 888 mAh g−1 at 0.5 C and shows a slow capacity decay rate of 0.025%/cycle after 200 cycles. Even when the areal loading of active sulfur is added up to 5 mg cm−2, the battery can also show a stable cycle performance for more than 300 cycles." @default.
• W3150596379 created "2021-04-13" @default.
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• W3150596379 date "2021-06-01" @default.
• W3150596379 modified "2023-10-18" @default.
• W3150596379 title "Co-N/KB porous hybrid derived from ZIF 67/KB as a separator modification material for lithium-sulfur batteries" @default.
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• W3150596379 doi "https://doi.org/10.1016/j.electacta.2021.138282" @default.
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