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- W3150607206 abstract "Abstract Transition-metal-catalyzed nucleophilic C–H addition of hydrocarbons to polar unsaturated bonds could intrinsically avoid prefunctionalization of substrates and formation of waste byproducts, thus featuring high step- and atom-economy. As the third most abundant transition metal, manganese-catalyzed C–H addition to polar unsaturated bonds remains challenging, partially due to the difficulty in building a closed catalytic cycle of manganese. In the past few years, we have developed manganese catalysis to enable the sp2-hydrid C–H addition to polar unsaturated bonds (e.g., imines, aldehydes, nitriles), which will be discussed in this personal account. 1 Introduction 2 Mn-Catalyzed N-Directed C(sp2)–H Addition to Polar Unsaturated Bonds 3 Mn-Catalyzed O-Directed C(sp2)–H Addition to Polar Unsaturated Bonds 4 Conclusion" @default.
- W3150607206 created "2021-04-13" @default.
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- W3150607206 date "2021-03-27" @default.
- W3150607206 modified "2023-10-18" @default.
- W3150607206 title "Manganese-Catalyzed C(sp2)–H Addition to Polar Unsaturated Bonds" @default.
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- W3150607206 doi "https://doi.org/10.1055/a-1468-6136" @default.
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