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- W3153979427 abstract "Engineering symmetry breaking in seed-mediated growth is a fundamental challenge to produce colloidal nanocrystals with controlled morphologies and properties. In this work, we show a simple, aqueous approach to breaking the inversion symmetry of silver nanorods by restricting growth to one end of the pentatwinned gold bipyramid seed. Controlled addition of dimethyl sulfoxide (DMSO) allows us to tune both the symmetry and the length and width of the objects. Simulations and experiments demonstrate the adsorption of DMSO, which displaces interfacial water, reduces binding of surfactant and chloride ions at the gold surface, and slows down the deposition kinetics of silver. Besides showing the potential of DMSO for controlling the synthesis of complex nanostructures, this work opens new perspectives for the study of the physical properties of noncentrosymmetric nanoparticles, e.g., by controlling their plasmon modes and their second-harmonic generation efficiency." @default.
- W3153979427 created "2021-04-26" @default.
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- W3153979427 date "2021-04-16" @default.
- W3153979427 modified "2023-10-05" @default.
- W3153979427 title "Symmetry Breaking in Seed-Mediated Silver Nanorod Growth Induced by Dimethyl Sulfoxide" @default.
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- W3153979427 doi "https://doi.org/10.1021/acs.chemmater.1c00454" @default.
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