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• W3154268532 abstract "Mineral carbonation in an aqueous solution is one of the practical strategies in carbon capture utilization and storage (CCUS). The wet carbonation can be further used to produce calcium carbonate nanoparticles with vast applications. Since the slow CO2 absorption affects the carbonation reaction, membrane gas absorption (MGA) with porous membranes was used in this study to enhance the mass transfer of CO2 gas into liquid absorbent for the carbonation of calcium-rich solution. The effects of sodium dodecyl sulphates (SDS) and poly(ethylene glycol) (PEG) on the properties of CaCO3 nanoparticles formed in wet carbonation were first studied. The calcite nanoparticles with particle size smaller than 25 nm were successfully produced, as proven in X-ray diffraction analysis and the transmission electron microscope images. Calcite nanoparticles with a BET surface area of 77.17 m2/g could adsorb 91.8 % of Congo red dye. The wet carbonation with surfactant-template was subsequently integrated with MGA. The pure CO2 absorption flux through the silanized polyvinylidene fluoride (PVDF)/TiO2 membrane enabled the formation of calcite nanoparticles in a calcium-rich solution containing a surfactant-template complex. The slow CO2 absorption flux of the commercial PVDF membrane with a hydrophobic surface cause failure to produce calcite with nano size." @default.
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• W3154268532 date "2021-06-01" @default.
• W3154268532 modified "2023-10-18" @default.
• W3154268532 title "Carbon dioxide conversion into calcium carbonate nanoparticles using membrane gas absorption" @default.
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• W3154268532 doi "https://doi.org/10.1016/j.jcou.2021.101533" @default.
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