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• W3154722734 endingPage "159964" @default.
• W3154722734 startingPage "159964" @default.
• W3154722734 abstract "• Centimeter-level Dy-based bulk metallic glass was prepared through microalloying Si element. • The nucleation is suppressed with 1 at% Si addition while accelerated with 3 at% Si addition. • The precipitates grow slowly for Dy 55 Co 20 Al 24 Si 1 BMG whereas rapidly for Dy 55 Co 20 Al 22 Si 3 BMG. • Thermodynamic and kinetic properties show non-linear variation with increasing Si content. In this work, the glass-forming ability of DyCoAl bulk metallic glass (BMG) was improved by microalloying Si element. Centimeter-level Dy-based BMG was prepared with the addition of 1 at% Si at the expense of Al element. Distinctions of crystallization behavior induced by Si addition for the Dy 55 Co 20 Al 25 BMG were investigated in terms of isochronal and isothermal crystallization as well as time dependent crystallization. Compared with the Dy 55 Co 20 Al 25 BMG, the nucleation process changes to a suppressed nucleation with 1 at% Si addition, and then to an explosive nucleation with 3 at% Si addition accompanying the precipitation of Si-containing phases. Meanwhile, the growth of crystalline particle is sluggish for Dy 55 Co 20 Al 24 Si 1 BMG whereas turns to rapid for Dy 55 Co 20 Al 22 Si 3 BMG. These distinctions of crystallization behavior are attributed to the interplay of driving force for crystallization and kinetic fragility of supercooled liquid. This work provides guidance to modulate the magnetocaloric effect of Dy-based BMGs through crystallization treatment." @default.
• W3154722734 created "2021-04-26" @default.
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• W3154722734 date "2021-09-01" @default.
• W3154722734 modified "2023-10-02" @default.
• W3154722734 title "Effects of Si addition on glass-forming ability and crystallization behavior of DyCoAl bulk metallic glass" @default.
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• W3154722734 doi "https://doi.org/10.1016/j.jallcom.2021.159964" @default.
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