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- W3157029107 abstract "A new access to artemisinin is reported based on a selective photochemical hydrothiolation of amorphadiene, a waste product of the industrial semisynthetic route. This study highlights the discovery of two distinctive activation pathways under solvent-free conditions or using a photocatalyst promoting H-abstraction. Subsequently, a chemoselective oxidation of the resulting photochemically generated thioether, followed by a Pummerer rearrangement, affords dihydroartemisinic aldehyde, a key intermediate in the synthesis of artemisinin." @default.
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- W3157029107 date "2021-04-26" @default.
- W3157029107 modified "2023-10-14" @default.
- W3157029107 title "Photochemical Hydrothiolation of Amorphadiene and Formal Synthesis of Artemisinin via a Pummerer Rearrangement" @default.
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- W3157029107 doi "https://doi.org/10.1021/acs.orglett.1c00636" @default.
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