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• W3157135685 abstract "Isoreticular functionalization is a well-elucidated strategy for pore environment tuning and the basis of gas separation performance in extended frameworks. The extension of this approach to discrete porous molecules such as metal-organic cages (MOCs) is conceptually straightforward but hindered by synthetic complications, especially stability concerns. We report the successful isoreticular functionalization of a zirconium MOC with tetrazole moiety by bottom-up synthesis. The title compound (ZrT-1-tetrazol) shows promising C2H2/CO2 and C2H2/C2H4 separation performance, as demonstrated by adsorption isotherms, breakthrough experiments, and density functional theory calculations. The design analogy between MOFs and highly stable MOCs may guide the synthesis of novel porous materials for challenging separation applications." @default.
• W3157135685 created "2021-05-10" @default.
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• W3157135685 date "2021-06-14" @default.
• W3157135685 modified "2023-10-17" @default.
• W3157135685 title "Tetrazole‐Functionalized Zirconium Metal‐Organic Cages for Efficient C ₂ H ₂ /C ₂ H ₄ and C ₂ H ₂ /CO ₂ Separations" @default.
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• W3157135685 doi "https://doi.org/10.1002/anie.202102585" @default.
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