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- W3157231855 abstract "Abstract Organosilicon compounds are important reagents and synthetic intermediates that play a key role in the construction of new materials and complex products. Here we show a highly diastereoselective rhodium‐catalyzed cycloisomerization of 1,6‐dienes, in which the use of (EtO) 3 SiH accelerates the intramolecular cyclization reaction to afford a novel spiro‐fused succinimide and pyrazolone derivatives in moderate to excellent yields as a single diastereoisomer. The proposed mechanism involves an active Rh−H species from the hydrosilane that is the H‐donor in this spiro‐type cycloisomerization reaction." @default.
- W3157231855 created "2021-05-10" @default.
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- W3157231855 date "2021-05-18" @default.
- W3157231855 modified "2023-10-12" @default.
- W3157231855 title "Highly Diastereoselective Hydrosilane‐Assisted Rhodium‐Catalyzed Spiro‐Type Cycloisomerization of Succinimide and Pyrazolone‐Based Functional 1,6‐Dienes" @default.
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- W3157231855 doi "https://doi.org/10.1002/asia.202100372" @default.
- W3157231855 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33945231" @default.
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