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- W3157396108 abstract "• Carbon quantum dots-modified reduced ultrathin g-C 3 N 4 (RUCN/CQD) was prepared with facile method. • The RUCN/CQD possessed enhanced photoresponse and photoredox activities. • The RUCN/CQD exhibited superior photocatalytic activities in simulated natural conditions. Graphitic carbon nitride (g-C 3 N 4 ) has been extensively applied for the photocatalytic degradation of pharmaceuticals and personal care products (PPCPs); however, its catalytic performance remains restricted by a poor photoresponse and modest photoredox capacity toward the generation of free radicals. Herein, a novel carbon quantum dots-modified reduced ultrathin g-C 3 N 4 (RUCN/CQD) photocatalyst was successfully synthesized, with the capacity for direct •OH and O 2 •− yields and a broad-spectrum response. Upon broad-spectrum light irradiation, the RUCN/CQD demonstrated a 100% removal rate for diclofenac (DCF) within six min. This remarkable performance was attributed to a customized band structure with a thermodynamic driving potential for the generation of •OH, CQD with an effective electron transfer capacity for promotional formation of O 2 •− , and ultrathin porous structure with abundant reaction sites. Simultaneously, the up-converted fluorescent properties of the CQD endowed the photocatalyst with a broad-spectrum response. The RUCN/CQD system also exhibited superior photocatalytic activities under simulated natural conditions, which implied an immense potential for the remediation of PPCPs in ambient waterways." @default.
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- W3157396108 date "2021-09-01" @default.
- W3157396108 modified "2023-10-10" @default.
- W3157396108 title "Carbon quantum dots-modified reduced ultrathin g-C3N4 with strong photoredox capacity for broad spectrum-driven PPCPs remediation in natural water matrices" @default.
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- W3157396108 doi "https://doi.org/10.1016/j.cej.2021.129935" @default.
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