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- W3157447670 abstract "Herein, we report the first example of covalent organic framework (DHBD-TMT) linked by unsubstituted olefin-linkages for selective loading, chemical reduction and photocatalytic reduction of uranium. The unique structures of DHBD-TMT possess all the characteristics to be well suited as a capture platform for selective ligand complexation, efficient chemical reduction and photocatalytic reduction of uranium, thus exhibiting a groundbreaking uranium capture capacity (2640.8 mg g-1). In the dark, DHBD-TMT can effectively adsorb uranium through the hydroxyl groups laced on the skeleton and reduce UVI to UIV in situ, leading to a higher adsorption capacity and selectivity of uranium. At the same time, the synergistic effect of the hydroquinone and triazine units in the extended π-conjugated skeleton significantly improve the photocatalytic activity of DHBD-TMT, and an additional UVI photocatalytic reduction mechanism can occur under visible light irradiation, allowing significantly higher the capacity and faster adsorption kinetics." @default.
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- W3157447670 date "2021-10-01" @default.
- W3157447670 modified "2023-10-18" @default.
- W3157447670 title "Rational design of covalent organic frameworks as a groundbreaking uranium capture platform through three synergistic mechanisms" @default.
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- W3157447670 doi "https://doi.org/10.1016/j.apcatb.2021.120250" @default.
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