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• W3157562222 endingPage "4075" @default.
• W3157562222 startingPage "4075" @default.
• W3157562222 abstract "Degradation models are commonly used to describe the generation of combustible gases when predicting fire behavior. A model may include many sub-models, such as heat and mass transfer models, pyrolysis models or mechanical models. The pyrolysis sub-models require the definition of a decomposition mechanism and the associated reaction rates. Arrhenius-type equations are commonly used to quantify the reaction rates. Arrhenius-type equations allow the representation of chemical decomposition as a function of temperature. This representation of the reaction rate originated from the study of gas-phase reactions, but it has been extrapolated to liquid and solid decomposition. Its extension to solid degradation needs to be justified because using an Arrhenius-type formulation implies important simplifications that are potentially questionable. This study describes these simplifications and their potential consequences when it comes to the quantification of solid-phase reaction rates. Furthermore, a critical analysis of the existing thermal degradation models is presented to evaluate the implications of using an Arrhenius-type equation to quantify mass-loss rates and gaseous fuel production for fire predictions." @default.
• W3157562222 created "2021-05-10" @default.
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• W3157562222 date "2021-04-29" @default.
• W3157562222 modified "2023-10-05" @default.
• W3157562222 title "Origin and Justification of the Use of the Arrhenius Relation to Represent the Reaction Rate of the Thermal Decomposition of a Solid" @default.
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• W3157562222 doi "https://doi.org/10.3390/app11094075" @default.
• W3157562222 hasPublicationYear "2021" @default.
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