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• W3157628384 abstract "• Metal ions inhibit Hg 0 re-emission under air and oxy-fuel combustion atmospheres. • The mechanisms were explored through mercury re-emission and migration behaviors. • Metal ions can promote mercury stabilization in liquid and solid phases. • The impacts of O 2 and CO 2 are distinct in the presence of different metal ions. The effects of metal ions, including Fe 2+ , Fe 3+ , Mn 2+ , and Cu 2+ , on Hg 0 re-emission were investigated in a simulated wet flue gas desulfurization (WFGD) system under air and oxy-fuel combustion atmospheres. The results show that in the presence of metal ions, Hg 0 re-emission is enhanced under a N 2 atmosphere but inhibited under N 2 /9%O 2 , air, and oxy-fuel combustion atmospheres. In the inhibition cases, Hg 2+ reduction and Hg 0 re-emission were accelerated in the initial stages of the experiments. Fortunately, Fe 2+ , Fe 3+ , Mn 2+ , and Cu 2+ have a positive impact on mercury stabilization in the liquid phase, and the precipitates of Fe 2+ /Fe 3+ can also adsorb mercury in the solid phase, thus offsetting the acceleration of Hg 0 re-emission in the initial stage. Therefore, Hg 0 re-emission is suppressed by metal ions under N 2 /9%O 2 , air, and oxy-fuel combustion atmospheres. With an increase in CO 2 concentration, the inhibition of Fe 2+ , Fe 3+ , and Cu 2+ was intensified, whereas the suppression by Mn 2+ was slightly weakened. Under an oxy-fuel combustion atmosphere, increasing O 2 concentration would promote the inhibition of Mn 2+ on Hg 0 re-emission, but hardly affect the inhibitory effect of Cu 2+ ." @default.
• W3157628384 created "2021-05-10" @default.
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• W3157628384 date "2021-09-01" @default.
• W3157628384 modified "2023-10-16" @default.
• W3157628384 title "Effects of metal ions on Hg0 re-emission under air and oxy-fuel combustion atmospheres in a WFGD system" @default.
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• W3157628384 doi "https://doi.org/10.1016/j.fuel.2021.120881" @default.
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