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• W3157782626 endingPage "106081" @default.
• W3157782626 startingPage "106081" @default.
• W3157782626 abstract "Hydrodeoxygenation of lipids is a promising method to produce diesel-like hydrocarbons. In this work, NiO/TS-1 and Ni/TS-1 catalysts were synthesized, and the catalytic hydrodeoxygenation of palmitic acid to produce diesel-like hydrocarbons was investigated. The effect of reaction time (2–10 h) and H 2 pressure (1–5 MPa) on the production of diesel-like hydrocarbons were also studied in detail. Finally, a possible reaction route was proposed. The results showed that catalytic hydrodeoxygenation performance is affected by the valence of active component Ni. Ni/TS-1 shows better catalytic performance than NiO/TS-1 in terms of palmitic acid conversion and alkanes selectivity. Under the optimal experimental conditions (260 °C, 4 MPa, 10 h, 400 rpm), the palmitic acid conversion and pentadecane selectivity over Ni/TS-1 are 100% and 91.6%, respectively. It is found that hexadecanol is an important intermediate in the hydrodeoxygenation of palmitic acid. • The valence of nickel strongly affects conversion of palmitic acid and selectivity of diesel-like hydrocarbons. • Ni/TS-1 was used for hydrodeoxygenation of palmitic acid to produce diesel-like alkanes. • 100% conversion of palmitic acid and 91.6% selectivity of pentadecane could be obtained over Ni/TS-1. • Hexadecanol is a key intermediate during the hydrodeoxygenation of palmitic acid. • Decarbonylation is the main route for the hydrodeoxygenation of palmitic acid over Ni/TS-1 catalyst." @default.
• W3157782626 created "2021-05-10" @default.
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• W3157782626 date "2021-06-01" @default.
• W3157782626 modified "2023-10-18" @default.
• W3157782626 title "Production of diesel-like hydrocarbons via hydrodeoxygenation of palmitic acid over Ni/TS-1 catalyst" @default.
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• W3157782626 doi "https://doi.org/10.1016/j.biombioe.2021.106081" @default.
• W3157782626 hasPublicationYear "2021" @default.
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