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• W3157957306 abstract "The reduction of carbon dioxide (CO2 ) into value-added fuels using an electrochemical method has been regarded as a compelling sustainable energy conversion technology. However, high-performance electrocatalysts for CO2 reduction reaction (CO2 RR) with high formate selectivity and good stability need to be improved. Earth-abundant Bi has been demonstrated to be active for CO2 RR to formate. Herein, we fabricated an extremely active and selective bismuth nanosheet (Bi-NSs) assembly via an in situ electrochemical transformation of (BiO)2 CO3 nanostructures. The as-prepared material exhibits high activity and selectivity for CO2 RR to formate, with nearly 94% faradaic efficiency at -1.03 V (versus reversible hydrogen electrode (vs. RHE)) and stable selectivity (>90%) in a large potential window ranging from -0.83 to -1.18 V (vs. RHE) and excellent durability during 12 h continuous electrolysis. In addition, the Bi-NSs based CO2 RR/methanol oxidation reaction (CO2 RR/MOR) electrolytic system for overall CO2 splitting was constructed, evidencing the feasibility of its practical implementation." @default.
• W3157957306 created "2021-05-10" @default.
• W3157957306 creator A5026605210 @default.
• W3157957306 creator A5036344147 @default.
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• W3157957306 creator A5051155849 @default.
• W3157957306 date "2021-05-10" @default.
• W3157957306 modified "2023-10-10" @default.
• W3157957306 title "<i>In Situ</i> Bismuth Nanosheet Assembly for Highly Selective Electrocatalytic CO ₂ Reduction to Formate" @default.
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• W3157957306 doi "https://doi.org/10.1002/asia.202100305" @default.
• W3157957306 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33929102" @default.
• W3157957306 hasPublicationYear "2021" @default.
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