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• W3158187263 abstract "• A dual Z-scheme AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 heterojunction was designed. • AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 composite showed superior photodegradation of RhB and TC. • 1T-2H MoSe 2 between AgI and Bi 4 O 5 Br 2 serves as an interfacial charge transfer bridge across dual Z-scheme junction. • Band offsets were introduced in photocatalytic mechanism of AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 . • 1T-2H MoSe 2 bridged dual Z-scheme MoSe 2 -based heterojunction mechanism was proposed. The transition-metal dichalcogenides (TMDs) with 1T phase structure holds great promise for providing abundant active sites and superior conductivity, while the achievement of highly efficient degradation activity over bare TMDs and TMDs-based photocatalysts is still challenges. In this work, a flower-like mixed 1T-2H phase MoSe 2 was synthesized via a sodium borohydride (NaBH 4 )-assisted solvothermal method, and then was selected as a “charge-transfer-bridge” to fabricate a dual Z-scheme AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 composite with a 0D/3D hierarchical structure. The optimal AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 composite exhibited the superior photocatalytic activity towards degrading RhB and TC relative to AgI/2H MoSe 2 /Bi 4 O 5 Br 2 and AgI/Bi 4 O 5 Br 2 . The enhancement is attributed to its better light absorption, abundant active sites, and superior charge carrier mobility and separation efficiency, resulted from synergetic effect of 0D/3D structural coupling and energy band matching. Moreover, the important energy band alignments and mixed 1T-2H phase MoSe 2 boosting photocatalytic mechanism of as-prepared AgI/1T-2H MoSe 2 /Bi 4 O 5 Br 2 heterojunction were investigated. This work describes a competitive design and fabrication technique for constructing novel mixed phase TMDs-based Z-scheme heterojunctions to address environmental issues." @default.
• W3158187263 created "2021-05-10" @default.
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• W3158187263 date "2021-09-01" @default.
• W3158187263 modified "2023-10-18" @default.
• W3158187263 title "Mixed 1T-2H phase MoSe2 as interfacial charge-transfer-bridge to boosting photocatalytic activity of dual Z-scheme AgI/1T-2H MoSe2/Bi4O5Br2 heterojunction" @default.
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• W3158187263 doi "https://doi.org/10.1016/j.jallcom.2021.160092" @default.
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