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• W3159376980 abstract "Insufficient active sites and fast charge carrier recombination are detrimental to photocatalytic activity of graphitic carbon nitride (g-C3N4). In this work, a combination of pore creating with thermal exfoliation was employed to prepare porous g-C3N4 nanosheets for photocatalytic water splitting into hydrogen. Hexadecyl trimethyl ammonium chloride (CTAC) as the soft template promoted the formation of porous g-C3N4 during the thermal condensation of melamine. On further post-synthesis calcination, the porous g-C3N4 aggregates were exfoliated into discrete nanosheets, accompanied by an increase in specific surface area and defects. Optimal porous g-C3N4 nanosheets achieved 3.6 times the photocatalytic hydrogen evolution rate for bulk counterpart. The enhanced photocatalytic activity may be ascribed to TCN-1%CTAC has larger specific surface area, stronger optical absorption intensity and higher photogenerated electron–hole separation efficiency. The external quantum efficiency of TCN-1%CTAC was measured to be 3.4% at 420 nm. This work provides a simple combinatorial strategy for the preparation of porous g-C3N4 nanosheets with low cost, environmental friendliness and enhanced photocatalytic activity." @default.
• W3159376980 created "2021-05-10" @default.
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• W3159376980 date "2021-07-01" @default.
• W3159376980 modified "2023-10-17" @default.
• W3159376980 title "Combined soft templating with thermal exfoliation toward synthesis of porous g-C3N4 nanosheets for improved photocatalytic hydrogen evolution" @default.
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• W3159376980 doi "https://doi.org/10.1016/j.jmrt.2021.04.056" @default.
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