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- W3159432967 abstract "A prevailing perception on Mg metal anodes is that high ion-diffusion barriers in corresponding passivated interfaces can induce poor reversibility and high overpotential. However, the dynamic evolution and degradation of native solid/electrolyte interfaces (SEI) in the electrochemical process has not yet been established. To unravel the origin of unstable Mg anodes, this study comprehensively reveals the native SEI is dominated by organic components. A model system with controllable electronically insulating SEI is designed by increasing the inorganic component, to provide a new insight that the interfacial electronic property and composition is decisive to the degradation of Mg metal anodes. The initial organic-rich SEI with insufficient electrical insulation in turn hinders ion transport by undergoing continuous cracking/reformation and electronic leakage which induces continuous proliferation during operation process. By optimizing electronic insulation of the initial interface, a symmetric cell exhibits superior cycling performances of over 1150 h with low polarization." @default.
- W3159432967 created "2021-05-10" @default.
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- W3159432967 date "2021-08-01" @default.
- W3159432967 modified "2023-10-18" @default.
- W3159432967 title "Revisiting the degradation of solid/electrolyte interfaces of magnesium metal anodes: Decisive role of interfacial composition" @default.
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- W3159432967 doi "https://doi.org/10.1016/j.nanoen.2021.106087" @default.
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